I don't think it has to be one or the other...both have benefits, especially if you are working up to a goal such as a long-distance race. Doing two 30 minute sessions will allow you to push more intensely each time and burn more calories both during and after the workout. However, one 60 minute session allows you to challenge yourself cardiovascularly and helps your lung efficiency. Additionally, doing both types of workouts each week keeps your body constantly challenged. I would try doing one of each per week, plus the other 35 minute workouts you described.